Self-Assembled Film Organization in Fast Microcontact Printing Investigated by Sum Frequency Generation Spectroscopy

[en] The ability of microcontact printing to build highly ordered alkanethiol self-assembled monolayers (SAMs) on Pt substrates within a short time is studied by sum frequency generation (SFG) spectroscopy and contact angle measurements. The deposition of ordered hexadecanethiol and dodecanethiol monolayers onto platinum substrates is achieved in less than 1 s. The film order and the alkane chain orientation are deduced from the SFG fingerprint acquired under different sets of laser polarization. Comparisons between the SAMs prepared by printing or by immersion demonstrate that both methods lead to the same high quality organization. Patterning effects within printed films are also investigated with respect to the layer conformation. Finally, wetting properties of printed layers are correlated with the printing duration, corroborating the spectroscopic results.

Disciplines :

Physics

Author, co-author :

Lis, Dan

Peremans, André

Sartenaer, Yannick

Caudano, Yves

Mani, Alaa Addin

Dreesen, Laurent ; Université de Liège - ULiège > Département de physique > Biophotonique

Thiry, Paul A.

Guthmuller, Julien

Champagne, Benoît

Cecchet, Francesca

Language :

English

Title :

Self-Assembled Film Organization in Fast Microcontact Printing Investigated by Sum Frequency Generation Spectroscopy

Publication date :

2009

Journal title :

Journal of Physical Chemistry. C, Nanomaterials and interfaces

ISSN :

1932-7447

eISSN :

1932-7455

Publisher :

American Chemical Society, Washington, United States - District of Columbia

Volume :

113

Pages :

9857-9864

Peer reviewed :

Peer Reviewed verified by ORBi

Available on ORBi :

since 26 October 2009

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