Enhanced Debye level in nano Zn1+xSb, FeSb2, and NiSb: Nuclear inelastic spectroscopy on121 Sb

Claudio, T.; Bessas, D.; Birke, C. S.; Kieslich, G.; Panthöfer, M.; Sergueev, I.; Tremel, W.; Hermann, Raphaël

doi:10.1002/pssb.201350246

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Enhanced Debye level in nano Zn1+xSb, FeSb2, and NiSb: Nuclear inelastic spectroscopy on121 Sb

Claudio, T.; Bessas, D.; Birke, C. S. et al.

2014 • In Physica Status Solidi B. Basic Research, 251 (5), p. 919-923

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10.1002/pssb.201350246

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Keywords :

Antimonides; Density of phonon states; Nanoparticles; Nuclear inelastic scattering

Abstract :

[en] The121 Sb partial density of phonon states (DPS) in nanopowder antimonides were obtained with nuclear inelastic scattering on Zn1+xSb, FeSb2, and NiSb prepared by a wet chemistry route. The DPS is compared with the bulk counterpart. An increase of the Debye level indicative of a decrease of the isothermal speed of sound is systematically observed. This observation reveals that the decrease in speed of sound observed in nanostructured thermoelectric materials is not restricted to sintered nanocomposites. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Disciplines :

Physics

Author, co-author :

Claudio, T.; Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, 52425 Jülich, Germany, Faculté des Sciences, Université de Liège, 4000 Liège, Belgium

Bessas, D.; Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, 52425 Jülich, Germany, Faculté des Sciences, Université de Liège, 4000 Liège, Belgium, European Synchrotron Radiation Facility, 38043 Grenoble Cedex, France

Birke, C. S.; Institut für Anorganische Chemie und Analytische Chemie der Johannes Gutenberg-Universität, Duesbergweg 10-14, 55099 Mainz, Germany, Materials Research Laboratory, University of California, Santa Barbara, CA, United States

Kieslich, G.; Institut für Anorganische Chemie und Analytische Chemie der Johannes Gutenberg-Universität, Duesbergweg 10-14, 55099 Mainz, Germany

Panthöfer, M.; Institut für Anorganische Chemie und Analytische Chemie der Johannes Gutenberg-Universität, Duesbergweg 10-14, 55099 Mainz, Germany

Sergueev, I.; Jülich Centre for Neutron Science JCNS, Peter Grünberg Institut PGI, JARA-FIT, Forschungszentrum Jülich GmbH, 52425 Jülich, Germany, European Synchrotron Radiation Facility, 38043 Grenoble Cedex, France

Tremel, W.; Institut für Anorganische Chemie und Analytische Chemie der Johannes Gutenberg-Universität, Duesbergweg 10-14, 55099 Mainz, Germany

Hermann, Raphaël ; Université de Liège > Département de chimie (sciences) > Département de chimie (sciences)

Language :

English

Title :

Enhanced Debye level in nano Zn1+xSb, FeSb2, and NiSb: Nuclear inelastic spectroscopy on121 Sb

Publication date :

2014

Journal title :

Physica Status Solidi B. Basic Research

ISSN :

0370-1972

eISSN :

1521-3951

Publisher :

Wiley-VCH Verlag

Volume :

251

Issue :

Pages :

919-923

Peer reviewed :

Peer Reviewed verified by ORBi

Available on ORBi :

since 01 June 2015

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