References of "Remacle, Françoise"
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See detailMicrofluidic chip with molecular beacons detects miRNAs in Human CSF to reliably characterize CNS-specific disorders
Zadran, S.; Remacle, Françoise ULg; Levine, R. D.

in RNA & Disease (2016), 3

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See detailProbing in Space and Time the Nuclear Motion Driven by Nonequilibrium Electronic Dynamics in Ultrafast Pumped N2
Ajay, J.; Šmydke, J.; Remacle, Françoise ULg et al

in Journal of Physical Chemistry A (2016), 120(19), 3335-3342

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See detailQuantum Nuclear Dynamics Pumped and Probed by Ultrafast Polarization Controlled Steering of a Coherent Electronic State in LiH
Nikodem, Astrid ULg; Levine, R. D.; Remacle, Françoise ULg

in Journal of Physical Chemistry A (2016), 120(19), 3343-3352

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See detailTechniques for modulating error resilience in emerging multi-value technologies
Sjalander, Magnus; Borgstr, Gustaf; Klymenko, Mykhailo ULg et al

in Proceedings of the ACM International Conference on Computing Frontiers (2016)

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See detailOperation of a quantum dot in the finite-state machine mode: Single-electron dynamic memory
Klymenko, Mykhailo ULg; Klein, M.; Levine, R. D. et al

in Journal of Applied Physics (2016), 120(2), 024503

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See detailControlling coherent quantum nuclear dynamics in LiH by ultra short IR atto pulses
Nikodem, Astrid ULg; Levine, R. D.; Remacle, Françoise ULg et al

in Progress in Ultrafast Laser Science XIII (2016)

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See detailExperimental and Theoretical Study of the Reactivity of Gold Nanoparticles Towards Benzimidazole-2-ylidene Ligands
Rodríguez-Castillo, María; Lugo-Preciado, Gustavo; Laurencin, Danielle et al

in Chem. Eur. J. (2016), 22

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See detailForce measurements reveal how small binders perturb the dissociation mechanisms of DNA duplex sequences
Burmistrova, Anastasia; Fresch, Barbara ULg; Sluysmans, Damien ULg et al

in Nanoscale (2016), 8

The force-driven separation of double-stranded DNA is crucial to the accomplishment of cellular pro- cesses like genome transactions. Ligands binding to short DNA sequences can have a local stabilizing or ... [more ▼]

The force-driven separation of double-stranded DNA is crucial to the accomplishment of cellular pro- cesses like genome transactions. Ligands binding to short DNA sequences can have a local stabilizing or destabilizing effect and thus severely affect these processes. Although the design of ligands that bind to specific sequences is a field of intense research with promising biomedical applications, so far, their effect on the force-induced strand separation has remained elusive. Here, by means of AFM-based single mole- cule force spectroscopy, we show the co-existence of two different mechanisms for the separation of a short DNA duplex and demonstrate how they are perturbed by small binders. With the support of Mole- cular Dynamics simulations, we evidence that above a critical pulling rate one of the dissociation pathways becomes dominant, with a dramatic effect on the rupture forces. Around the critical threshold, we observe a drop of the most probable rupture forces for ligand-stabilized duplexes. Our results offer a deep understanding of how a stable DNA–ligand complex behaves under force-driven strand separation [less ▲]

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See detailMetabolomic analysis of the green microalga Chlamydomonas reinhardtii cultivated under day/night conditions
Willamme, Rémi ULg; Alsafra, Zouheir; Arumugam, Rameshkumar et al

in Journal of Biotechnology (2015)

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See detailThe living of the green microalga Chlamydomonas reinhardtii in day/night cycles
Willamme, Rémi ULg; Alsafra, Zouheir; Alsafra, Rameshkumar et al

Poster (2015, March 13)

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See detailMeasurement and laser control of attosecond charge migration in ionized iodoacetylene
Kraus, P. M.; Mignolet, Benoît ULg; Baykusheva, D. et al

in Science (2015), 350(6262), 790-795

The ultrafast motion of electrons and holes after light-matter interaction is fundamental to a broad range of chemical and biophysical processes. We advanced high-harmonic spectroscopy to resolve ... [more ▼]

The ultrafast motion of electrons and holes after light-matter interaction is fundamental to a broad range of chemical and biophysical processes. We advanced high-harmonic spectroscopy to resolve spatially and temporally the migration of an electron hole immediately after ionization of iodoacetylene while simultaneously demonstrating extensive control over the process. A multidimensional approach, based on the measurement and accurate theoretical description of both even and odd harmonic orders, enabled us to reconstruct both quantum amplitudes and phases of the electronic states with a resolution of ~100 attoseconds. We separately reconstructed quasi–field-free and laser-controlled charge migration as a function of the spatial orientation of the molecule and determined the shape of the hole created by ionization. Our technique opens the prospect of laser control over electronic primary processes. [less ▲]

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See detailCharge Redistribution Effects on the UV-VIS Spectra of Small Ligated Gold Clusters: a Computational Study
Lugo Preciado, Jesus Gustavo ULg; Schwanen, Valérie ULg; Fresch, Barbara ULg et al

in Journal of Physical Chemistry C (2015), 119(20), 10969-10980

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See detailComputational benchmarking for ultrafast electron dynamics: wavefunction methods vs density functional theory
Oliveira, Micael J. T.; Mignolet, Benoît ULg; Kus, Tomasz et al

in Journal of Chemical Theory and Computation (2015), 11

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See detailMultivalley envelope function equations and effective potentials for phosphorus impurity in silicon
Klymenko, Mykhailo ULg; Rogge, S.; Remacle, Francoise ULg

in Physical Review B (2015), 92(19), 195302

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See detailInformation processing in parallel through directionally resolved molecular polarization components in coherent multidimensional spectroscopy
Yan, Tian-Min; Fresch, Barbara ULg; Levine, R. D. et al

in Journal of Chemical Physics (2015), 143(6), 064106

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See detailRelative Photoionization Cross Sections of Super-Atom Molecular Orbitals (SAMOs) in C60
Bohl, Elvira; Sokół, Katarzyna P.; Mignolet, Benoît ULg et al

in The Journal of Physical Chemistry A (2015), 119(47), 11504-11508

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See detailParallel and Multivalued Logic by the Two-Dimensional Photon-Echo Response of a Rhodamine–DNA Complex
Fresch, Barbara ULg; Cipolloni, Marco; Yan, Tian-Min ULg et al

in Journal of Physical Chemistry Letters (2015), 6

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See detailCoherent Electronic Wave Packet Motion in ${\mathrm{C}}_{60}$ Controlled by the Waveform and Polarization of Few-Cycle Laser Fields
Li, H.; Mignolet, Benoît ULg; Wachter, G. et al

in Physical Review Letters (2015), 114(12), 123004

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See detailTernary DNA computing using 3 x 3 multiplication matrices
Orbach, Ron; Lilienthal, Sivan; Klein, Michael et al

in Chemical Science (2015), 6

Non-Boolean computations implementing operations on multi-valued variables beyond base 2 allow enhanced computational complexity. We introduce DNA as a functional material for ternary computing, and in ... [more ▼]

Non-Boolean computations implementing operations on multi-valued variables beyond base 2 allow enhanced computational complexity. We introduce DNA as a functional material for ternary computing, and in particular demonstrate the use of three-valued oligonucleotide inputs to construct a 3 [times] 3 multiplication table. The system consists of two three-valued inputs of -1; 0; +1 and a fluorophore/quencher functional hairpin acting as computational and reporter module. The interaction of the computational hairpin module with the different values of the inputs yields a 3 [times] 3 multiplication matrix consisting of nine nanostructures that are read out by three distinct fluorescence intensities. By combining three different hairpin computational modules, each modified with a different fluorophore/quencher pair, and using different sets of inputs, the parallel operation of three multiplication tables is demonstrated. [less ▲]

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