References of "Piotrowska, Natalia"
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See detailHolocene dust record in a NW European peat bog: A multiproxy approach
Allan, Mohammed ULg; LE ROUX, gael; VERHEYDEN, SOPHIE et al

Conference (2013, August 28)

Dust deposition in southern Belgium is estimated from the geochemical signature of an ombrotrophic bog. The analyses of Rare Earth Elements (REE) and lithogenic element concentrations as well as Nd ... [more ▼]

Dust deposition in southern Belgium is estimated from the geochemical signature of an ombrotrophic bog. The analyses of Rare Earth Elements (REE) and lithogenic element concentrations as well as Nd isotopes were performed by HR-ICP-MS and MC-ICP-MS respectively, in a  6 m peat section representing 5300 years, from 30 BC to 5300 BC dated by the 14C method. REE concentration variations in peat samples were used as a dust proxy and the Nd isotopes to trace the sources. Peat humification and testate amoebae were used to evaluate hydroclimatic conditions. The range of dust deposition varied from 0.03 to 4 g m-2 yr-1. The highest dust fluxes were observed from 800 to 600 BC, and from 3200 to 2800 BC and correspond to cold periods. The Nd values show large variability, between -5 and –13, identifying three major sources of dust: local soils, distal volcanic and desert particles. By comparing our results with the dust recorded in other peat bogs and ice cores from different latitudes, we evidence that the Misten peat is a valid archive for dust deposition. [less ▲]

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See detailDust historical record in ombrotrophic peat: The case study of a NW European bog
Allan, Mohammed ULg; Fagel, Nathalie ULg; Le Roux, Gael et al

Poster (2013, May 16)

Ombrotrophic peatlands are unique environmental archives of natural and anthropogenic atmospheric dust deposition because their surface layers are exclusively fed by atmospheric inputs. Lead (Pb) isotopes ... [more ▼]

Ombrotrophic peatlands are unique environmental archives of natural and anthropogenic atmospheric dust deposition because their surface layers are exclusively fed by atmospheric inputs. Lead (Pb) isotopes have been often used to evidence any anthropogenic influence in peat, but they only record trace metal pollution. Another radiogenic isotope, the Neodymium (Nd), could be also use to discriminate the sources of dust in peat bogs. Dust fluxes were investigated over the last 2500 years in the Misten peat bog in Eastern Belgium. Our aims were to use Nd isotope signature to decipher between local and distal dust supplies, the Pb isotopes to trace the antropogenic influences. To address these aims we analyzed REE and lithogenic element analyses, as well as the Nd and Pb isotopes, using HR-ICP-MS and MC-ICP-MS, respectively in peat layers dated by 210Pb and 14C. Changes in REE concentration variations in peat samples are correlated with Ti, Al, and Zr that are lithogenic conservative elements, suggesting that REE are immobile in the studied peat bogs and can be used as tracers of dust deposition. Dust fluxes show pronounced increase at BC300, AD600, 1000AD, 1200AD and from 1700AD, recording either influence of human activities (regional erosion due to forest clearing and soil cultivation activities) or local and regional climate changes. Lead enrichments reveal strong human impact over the last 300 years. Lead isotope signatures are consistent with local and regional contamination by coal combustion and smelting activities. Neodymium isotopes allow to identify three periods characterised by dominant-distal sources (at 320AD, 1000 AD and 1700AD). Those periods are consistent with local wetter intervals as indicated by lower humification degree. Local erosion prevails durier drier (higher humification) intervals (-100AD, 600AD). On a global scale more distal supplies are driven during colder periods, in particular Oort and Maunder minima, confirming the hypothesis that cold climate conditions favor distal supplies. Combining geochemical elementary content and isotope data in ombrotrophic peat allows to decipher between dust flux changes related to human and climate forcing. [less ▲]

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See detailDeciphering human-climate interactions in ombrotrophic peat record : REE, Nd and Pb isotope signatures of dust supplies over the last 2500 years (Misten bog, Belgium)
Fagel, Nathalie ULg; Allan, Mohammed ULg; le roux, Gael et al

Poster (2013, April 08)

A core of 173 cm of ombrotrophic Misten peat bog from the Hautes-Fagnes Plateau in Eastern Belgium provides a record of Rare Earth Elements (REE) deposition allowing to trace dust fluxes in West Europe ... [more ▼]

A core of 173 cm of ombrotrophic Misten peat bog from the Hautes-Fagnes Plateau in Eastern Belgium provides a record of Rare Earth Elements (REE) deposition allowing to trace dust fluxes in West Europe during the historical record (last 2500 years). REE and lithogenic element analyses, as well as the Nd isotopes, were performed by HR-ICP-MS and MC-ICP-MS, respectively in peat layers dated by 210Pb and 14C. The parallel variations of REE concentration with lithogenic conservative elements confirms that REE are immobile in the studied peat bog and can be used as tracers of dust deposition. Dust fluxes show pronounced increase at BC300, AD600, 1000AD,1200AD and from 1700AD, recording either influence of human activities (regional erosion due to forest clearing and soil cultivation activities) or local and regional climate changes. Using Nd isotope allows to decipher between local and distal causes. The ENd variability (-13 to -9) is interpreted by a mixing between dust sources fromlocal soils and desert particles. Three periods characterised by dominant-distal sources (at 320AD, 1000 AD and 1700AD) are consistent with local wetter intervals as indicated by lower humi[U+FB01]cation degree. Local erosion prevails durier drier (higher humification) intervals (-100AD, 600AD). On a global scale more distal supplies are driven during colder periods, in particular Oort and Maunder minima. Combining geochemical elementary content and isotope data in ombrotrophic peat allows to decipher between dust flux changes related to human and climate forcing. [less ▲]

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See detailReconstructing historical atmospheric mercury deposition in Western Europe using: Misten peat bog cores, Belgium
Allan, Mohammed ULg; le roux, gael; E. Sonke, Jeroen et al

in Science of the Total Environment (2013), 442

Four sediment cores were collected in 2008 from the Misten ombrotrophic peat bog in the Northern part of the Hautes Fagnes Plateau in Belgium. Total mercury (Hg) concentrations were analyzed to ... [more ▼]

Four sediment cores were collected in 2008 from the Misten ombrotrophic peat bog in the Northern part of the Hautes Fagnes Plateau in Belgium. Total mercury (Hg) concentrations were analyzed to investigate the intra-site variability in atmospheric Hg deposition over the past 1500 years. Mercury concentrations in the four cores ranged from 16 to 1100 μg kg− 1, with the maxima between 840 and 1100 μg kg− 1. A chronological framework was established using radiometric 210Pb and 14C dating of two cores (M1 and M4). Pollen horizons from these two cores were correlated with data from two additional cores, providing a consistent dating framework between all the sites. There was good agreement between atmospheric Hg accumulation rates in the four cores over time based on precise age dating and pollen chronosequences. The average Hg accumulation rate before the influence of human activities (from 500 to 1300 AD) was 1.8 ± 1 μg m− 2 y− 1 (2SD). Maximum Hg accumulation rates ranged from 90 to 200 μg m− 2 y− 1 between 1930 and 1980 AD. During the European–North American Industrial Revolution, the mean Hg accumulation rate exceeded the pre-Industrial values by a factor of 63. Based on comparisons with historical records of anthropogenic activities in Europe and Belgium, the predominant regional anthropogenic sources of Hg during and after the Industrial Revolution were coal burning and smelter Hg emissions. Mercury accumulation rates and chronologies in the Misten cores were consistent with those reported for other European peat records. [less ▲]

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See detailHigh-resolution reconstruction of atmospheric deposition of trace metals and metalloids since AD 1400 recorded by ombrotrophic peat cores in Hautes-Fagnes, Belgium
Allan, Mohammed ULg; le roux, gael; De Vleeschouwer, François et al

in Environmental Pollution (2013), 1

The objective of our study was to determine the trace metal accumulation rates in the Misten bog, Hautes-Fagnes, Belgium, and assess these in relation to established histories of atmospheric emissions ... [more ▼]

The objective of our study was to determine the trace metal accumulation rates in the Misten bog, Hautes-Fagnes, Belgium, and assess these in relation to established histories of atmospheric emissions from anthropogenic sources. To address these aims we analyzed trace metals and metalloids (Pb, Cu, Ni, As, Sb, Cr, Co, V, Cd and Zn), as well as Pb isotopes, using XRF, Q-ICP-MS and MC-ICP-MS, respectively in two 40-cm peat sections, spanning the last 600 yr. The temporal increase of metal fluxes from the inception of the Industrial Revolution to the present varies by a factor of 5 to 50, with peak values found between AD 1930 and 1990. A cluster analysis combined with Pb isotopic composition allows the identification of the main sources of Pb and by inference of the other metals, which indicates that coal consumption and metallurgical activities were the predominant sources of pollution during the last 600 years. [less ▲]

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See detailMid and late Holocene dust deposition in Western Europe: The Misten peat bog (Hautes Fagnes - Belgium)
Allan, Mohammed ULg; Beghin, Jérémie ULg; le roux, Gael et al

in Climate of the Past (2013), 9(2889-2928,),

Dust deposition in southern Belgium is estimated from the geochemical signature of an ombrotrophic peatland. The Rare Earth Elements (REE) and lithogenic elements concentrations, as well as Nd isotopes ... [more ▼]

Dust deposition in southern Belgium is estimated from the geochemical signature of an ombrotrophic peatland. The Rare Earth Elements (REE) and lithogenic elements concentrations, as well as Nd isotopes, were determined by HR-ICP-MS and MC-ICP-MS respectively, along a  6 m peat section covering 5300 years, from 2000 to 7300 cal.BP dated by the 14C method. Changes in REE concentration in the peat correlate with those of Ti, Al, Sc and Zr that are lithogenic conservative elements, suggesting that REE are immobile in the studied peat bogs and can be used as tracers of dust deposition. Peat humification and testate amoebae were used to evaluate hydroclimatic conditions. The range of dust deposition varied from 0.03 to 4.0 g m-2 yr-1. The highest dust fluxes were observed from 2750 to 2550 cal.BP and from 5150 to 4750 cal.BP and correspond to cold periods. The Nd values show a large variability from -13 to –5, identifying three major sources of dusts: local soils, distal volcanic and desert particles. [less ▲]

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See detailMid and late Holocene dust deposition in Western Europe: The Misten peat bog (Hautes Fagnes - Belgium)
Allan, Mohammed ULg; Le Roux, Gael; Piotrowska, Natalia et al

Poster (2012, June)

Multi-proxy climate recorded from peatlands have been used to tracer the climate change during the Holocene. The initiation of peatland may be related to a change to colder and or wetter climate, and the ... [more ▼]

Multi-proxy climate recorded from peatlands have been used to tracer the climate change during the Holocene. The initiation of peatland may be related to a change to colder and or wetter climate, and the variations in peat composition reflect changes in precipitation and temperature. Peat has been used as an archive to reconstruct climate change over the Holocene (e.g., Shotyk et al., 1998; Sapkota et al., 2006). To characterize the climate in Belgium, a 570 cm-long core from Misten peat bog was studied. Several radiocarbon ages allow to define an accurate age model, the peat core represents 5500 years of record. The analyses of REE and lithogenic element contents, as well as the Nd isotopes, were performed by HR-ICP-MS and MC-ICP-MS. Peat humification, C/N ratio, ash content and bulk density were used to evaluate local hydroclimatic conditions. The dust deposition ranges from 0.03 to 4 g m -2 yr -1. As a first observation the highest rates of atmospheric dust deposition correspond to cold periods. The Nd values show large variability, between +1 to –22, identifying three major sources of dusts falling into the peat: local soils, distal volcanic and desert particles. Further studies are in progress to better identify the main forcing factor on the evolution of the atmospheric dust deposition over the Holocene. [less ▲]

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See detailAtmospheric mercury deposition during the last 1500 years in We Europe: The Misten peat bog record (Hautes Fagnes - Belgium)
Allan, Mohammed ULg; Fagel, Nathalie ULg; De Vleeschouwer, François et al

Poster (2011, April)

The current rate of global atmospheric Hg deposition is approximately three times higher than the preindustrial record and it even increased by a factor of 2-10 in the industrialized regions ... [more ▼]

The current rate of global atmospheric Hg deposition is approximately three times higher than the preindustrial record and it even increased by a factor of 2-10 in the industrialized regions.....()(Hylander and Meili 2003). To determine the extent of such increase, it is necessary to quantify the atmospheric mercury concentration and its temporal variation. For this purpose four 1m Wardenaar peat cores (MIS01W, 04W, 0W5 and 06W) were collected in 2008 in the ombrotrophic Misten bog (Hautes Fagnes Plateau, East Belgium). Mercury was measured using a DMA 80 at the Laboratory of Mechanisms and Transfers in Geology in Toulouse (LMTG, France). The strongest mercury concentrations are measured in the upper half peat record, in a depth interval corresponding to the Industrial Revolution period. Mercury accumulation rate was estimated by applying a coupled 210Pb- 14C age model. The mercury accumulation rate remains relatively small, ranging between 0.9 and 3.3 g.m 2.y 1 during periods corresponding to the decline of Roman Empire and during the Middle Ages. Hg accumulation rate starts to increase when 25 cm, reaching a maximum value (> 115 g.m 2.y 1) at 13.7 cm (i.e.; 1923-1938 AD). Then the values oscillate to reach 9 g.m 2.y 1 at the peat surface (2000-2007AD). In the Misten bog, the evolution of Hg accumulation rate is in agreement with the chronology of other European peat records .......()(Roos-Barraclough et al. 2002). [less ▲]

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See detailIntercomparison of radiocarbon bomb pulse and 210Pb age models. A study in a peat bog core from North Poland
Piotrowska, Natalia; De Vleeschouwer, François; Sikorski, Jaroslaw et al

in Nuclear Instruments & Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms (2010), Volume 268(7-8, April), 1163-1166

Radiocarbon and 210Pb were measured on the uppermost 40 cm of a Wardenaar peat core retrieved from a Baltic raised bog at Slowinskie Blota (Pomerania, North Poland). This site is the subject of ongoing ... [more ▼]

Radiocarbon and 210Pb were measured on the uppermost 40 cm of a Wardenaar peat core retrieved from a Baltic raised bog at Slowinskie Blota (Pomerania, North Poland). This site is the subject of ongoing multiproxy studies covering the last 1300 years. Radiocarbon age model was constructed on the basis of 14 AMS dates obtained on selected Sphagnum spp. fragments, with use of P_Sequence tool. We present here a comparison of this model with the age model obtained using CRS model classically applied to 210Pb measurements. [less ▲]

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See detailMutliproxy investigation of climatic and anthropogenic changes in a Baltic bog (N. Poland) during the last millennium
De Vleeschouwer, François; Fagel, Nathalie ULg; Piotrowska, Natalia et al

Poster (2010)

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See detailAnthropogenic impacts in North Poland over the last 1300 years -- A record of Pb, Zn, Cu, Ni and S in an ombrotrophic peat bog
De Vleeschouwer, François ULg; Fagel, Nathalie ULg; Cheburkin, Andriy et al

in Science of the Total Environment (2009)

Lead pollution history over Northern Poland was reconstructed for the last ca. 1300 years using the elemental and Pb isotope geochemistry of a dated Polish peat bog. The data show that Polish Pb–Zn ores ... [more ▼]

Lead pollution history over Northern Poland was reconstructed for the last ca. 1300 years using the elemental and Pb isotope geochemistry of a dated Polish peat bog. The data show that Polish Pb–Zn ores and coal were the main sources of Pb, other heavy metals and S over Northern Poland up until the industrial revolution. After review of the potential mobility of each element, most of the historical interpretation was based on Pb and Pb isotopes, the other chemical elements (Zn, Cu, Ni, S) being considered secondary indicators of pollution. During the last century, leaded gasoline also contributed to anthropogenic Pb pollution over Poland. Coal and Pb–Zn ores, however, remained important sources of pollution in Eastern European countries during the last 50 years, as demonstrated by a high 206Pb/207Pb ratio (1.153)relative to that of Western Europe (ca. 1.10). The Pb data for the last century were also in good agreement with modelled Pb inventories over Poland and the Baltic region. [less ▲]

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See detailMultiproxy evidence of `Little Ice Age' palaeoenvironmental changes in a peat bog from northern Poland
De Vleeschouwer, François ULg; Piotrowska, Natalia; Sikorski, Jaroslaw et al

in Holocene (2009), 19(4), 625-637

`Little Ice Age' (LIA) climatic deteriorations have been abundantly documented in various archives such as ice, lake sediments and peat bog deposits. Palaeoecological analyses of peat samples have ... [more ▼]

`Little Ice Age' (LIA) climatic deteriorations have been abundantly documented in various archives such as ice, lake sediments and peat bog deposits. Palaeoecological analyses of peat samples have identified these climatic deteriorations using a range of techniques, for example palynology, plant macrofossils, testate amoebae or carbon isotopic analyses. The use of inorganic geochemistry and the reconstruction of dust fluxes has remained a challenge in tracing the nature of LIA climatic changes. Although the idea of enhanced erosion conditions and storminess is commonly discussed, the conditions for dust deposition in peatlands over Europe during the LIA are rarely favourable, because the natural forest cover over Europe was much more important than nowadays, preventing dust deposition. This intense forest canopy masks the deposition of dust in peatlands. In northern Poland, near the Baltic shore, the S[l]owi[n]skie B[l]ota area was deforested around AD 1100, ie, just before the LIA, and therefore constitutes a key area for the reconstruction of LIA climatic change. With the support of a well-constrained chronology, climatic fluctuations are recorded in an ombrotrophic bog using inorganic geochemistry, plant macrofossils and carbon isotopic analyses. The reconstruction of LIA climatic changes is in good agreement with other records from Poland and NE Europe. However, a c. 50-year discrepancy can be observed between various records. This discrepancy is possibly due to progressive time-dependent cooling gradient from north to south Europe. [less ▲]

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See detailIntercomparison of lead 210 and radiocarbon bomb pulse age models. A key study in a peat bog core from North Poland
Piotrowska, Natalia; De Vleeschouwer, François; Sikorski, Jaroslaw et al

Poster (2008)

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See detailHigh-resolution diatom/clay record in Lake Baikal from grey scale, and magnetic susceptibility over Holocene and Termination I
Boes, Xavier; Piotrowska, Natalia; Fagel, Nathalie ULg

in Global and Planetary Change (2005), 46(1-4), 299-313

Tracing past climate signals from Lake Baikal sediments with a "multi-annual' resolution by conventional techniques is a difficult challenge since the sedimentation rates from Termination I up to the ... [more ▼]

Tracing past climate signals from Lake Baikal sediments with a "multi-annual' resolution by conventional techniques is a difficult challenge since the sedimentation rates from Termination I up to the present range from 0.004 to 0.17 mm/year. In this paper, climate signals are reconstructed from three continuous sediment records from Vydrino Shoulder and Posolsky Bank in the Southern Basin, and Continent Ridge in the Northern Basin. For each coring site, a calendar age model was constructed using calibrated radiocarbon ages. The magnetic susceptibility is used to better constrain the age models over OIS4 to OIS1 The cores have been hardened using polymerized technique in order to allow the easy cut of thin sections that contain evidence for narrow biogenic/clayey laminations. The grey scale taken from the thin sections is used here as a high-resolution proxy record of diatom/clay ratio. The grey density values are qualitatively interpreted against the sediment components by optical microscopy from the thin sections. In the Northern Basin, the Continent station provides the best age model and sediment resolution over the Termination I period. In particular, four optima (i.e. Bolling, Allerod, Atlantic, and Subboreal) are indicated by substantial increases of the grey scale, whereas cold periods like the Younger Dryas correspond to lower grey scale values. We emphasize that the short-term variations in the grey scale at 20 mu m resolution could correspond to short climate responses in Lake Baikal sediments. (C) 2004 Elsevier B.V. All rights reserved. [less ▲]

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