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See detailVolcano- and climate-driven changes in atmospheric dust sources and fluxes since the Late Glacial in Central Europe
Le Roux, Gael; Fagel, Nathalie ULg; De Vleeschouwer, François et al

in Geology (2012)

Atmospheric dusts are an important part of the global climate system, and play an important role in the marine and terrestrial bio- geochemical cycles of major and trace nutrient elements. A peat bog ... [more ▼]

Atmospheric dusts are an important part of the global climate system, and play an important role in the marine and terrestrial bio- geochemical cycles of major and trace nutrient elements. A peat bog record of atmospheric deposition shows considerable variation in dust deposition during the past 15 k.y., with abrupt changes in fl uxes at 12, 9.2, 8.4, 7.2, and 6 cal. kyr B.P. Using Nd isotopes and rare earth ele- ments, it is possible to clearly distinguish between volcanic inputs and those driven by climate change, such as the long-term aridifi cation of the Sahara and regional erosion due to forest clearing and soil cultiva- tion activities. Our results indicate that a major dust event in North Africa and Europe preceded the 8.2 kyr B.P. cold event by 200 yr. This dust event may have played an active role in the following climate cooling of the 8.2 kyr B.P. event. Nd isotope evidence also indicates a relatively slow change in dust regime over Europe from 7 to 5 kyr B.P. due to Sahara expansion. These fi ndings show that the inorganic frac- tion in high-resolution peat records can provide remarkably sensitive indicators of dust load and sources. Our study supports the priority to better identify the impact of dust loading during the Holocene in terms of direct and indirect impacts on environmental and climate changes. [less ▲]

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See detailHolocene evolution of deep circulation in the northern North Atlantic traced by Sm, Nd and Pb isotopes and bulk sediment mineralogy
Fagel, Nathalie ULg; Mattielli, Nadine ULg

in Paleoceanography (2011), 26

Bulk mineralogy, Sm, Nd and Pb elemental and isotopic compositions of the clay-size fraction of Holocene sediments were analysed in 3 deep North Atlantic cores to trace the particle provenance. The aims ... [more ▼]

Bulk mineralogy, Sm, Nd and Pb elemental and isotopic compositions of the clay-size fraction of Holocene sediments were analysed in 3 deep North Atlantic cores to trace the particle provenance. The aims of the present paper are to identify the origin of the particles driven by deep currents and to reconstruct deep circulation changes over the Holocene in the North Atlantic. The three cores are retrieved in fracture zones; two of them are located in the Island Basin along the gyre of North Atlantic Deep Water, and the third core is located off the present deep circulation gyre in the Labrador Sea. Whereas sedimentary supplies in the Labrador Sea were constantly derived from proximal sources, the geochemical mixing trends in the Iceland Basin samples indicate pronounced changes in the relative contribution of continental margin inputs over the past 6 kyr. Supplies from Western European margin that sharply increased at 6 kyr were progressively diluted by a larger contribution of Scandinavian margins over the last 3 kyr. Changes in composition of the particles imply significant reorganisation of paleocirculation of the deep North Atlantic components in the Eastern basins: mainly reorganisations for both Iceland-Scotland Overflow Water (ISOW) and Norwegian Sea Overflow Water (NSOW). Moreover the unusual Bulk mineralogy, Sm, Nd and Pb elemental and isotopic compositions of the clay-size fraction of Holocene sediments were analysed in 3 deep North Atlantic cores to trace the particle provenance. The aims of the present paper are to identify the origin of the particles driven by deep currents and to reconstruct deep circulation changes over the Holocene in the North Atlantic. The three cores are retrieved in fracture zones; two of them are located in the Island Basin along the gyre of North Atlantic Deep Water, and the third core is located off the present deep circulation gyre in the Labrador Sea. Whereas sedimentary supplies in the Labrador Sea were constantly derived from proximal sources, the geochemical mixing trends in the Iceland Basin samples indicate pronounced changes in the relative contribution of continental margin inputs over the past 6 kyr. Supplies from western European margin that sharply increased at 6 kyr were progressively diluted by a larger contribution of Scandinavian margins over the last 3 kyr. Changes in composition of the particles imply significant reorganisation of paleocirculation of the deep North Atlantic components in the eastern basins: mainly reorganisations for both Iceland-Scotland Overflow Water (ISOW) and Norwegian Sea Overflow Water (NSOW). Moreover the unusual Pb isotopic composition of the oldest sediments from the southern Iceland Basin indicates that distal supplies from Greenland margin were driven into the Iceland Basin, supporting a deep connection between Labrador Sea and Iceland Basin through the Charlie Gibbs Fracture Zone prior the Holocene Transition period. [less ▲]

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See detailAtmospheric lead and heavy metal pollution records from a Belgian peat bog spanning the last two millenia: Human impact on a regional to global scale
De Vleeschouwer, Francois; Gerard, Laetitia; Goormaghtigh, Catherine et al

in Science of the Total Environment (2007), 377(2-3), 282-295

Europe has been continuously polluted throughout the last two millennia. During the Roman Empire, these pollutions were mainly from ore extraction and smelting across Europe. Then, during the Middle Ages ... [more ▼]

Europe has been continuously polluted throughout the last two millennia. During the Roman Empire, these pollutions were mainly from ore extraction and smelting across Europe. Then, during the Middle Ages and the Early times of Industrial revolution (i.e. 1750), these pollutions extended to coal burning and combustion engine. Belgian ombrotrophic peat bogs have proved an effective archive of these pollutants and provide the opportunity to reconstruct the history of atmospheric deposition in NW Europe. The results of recent and past trace metal accumulation and Pb isotopes from a one-meter peat core (in the Misten peat bog) have been derived using XRF and Nu-plasma MC-ICP-MS. Combined with C-14 and Pb-210 dates these data have enabled us to trace fluxes in anthropogenic pollution back to original Roman times. Several periods of well-known Pb pollution events are clearly recorded including the Early and Late Roman Empire, the Middle Ages and the second industrial revolution. Also recorded is the introduction of leaded gasoline, and more recently the introduction of unleaded gasoline. Lead isotopes in this site have also enabled us to fingerprint several regional and global sources of anthropogenic particles. (c) 2007 Elsevier B.V. All rights reserved. [less ▲]

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