Use of second generation coated conductors for efficient shielding of DC magnetic fieldsFagnard, Jean-Francois ; ; et alin Journal of Applied Physics (2010), 108 This paper reports the results of an experimental investigation of the performance of two types of magnetic screens assembled from YBa2Cu3O7-d (YBCO) coated conductors. Since effective screening of the ... [more ▼] This paper reports the results of an experimental investigation of the performance of two types of magnetic screens assembled from YBa2Cu3O7-d (YBCO) coated conductors. Since effective screening of the axial DC magnetic field requires the unimpeded flow of an azimuthal persistent current, we demonstrate a configuration of a screening shell made out of standard YBCO coated conductor capable to accomplish that. The screen allows the persistent current to flow in the predominantly azimuthal direction at a temperature of 77 K. The persistent screen, incorporating a single layer of superconducting film, can attenuate an external magnetic field of up to 5 mT by more than an order of magnitude. For comparison purposes, another type of screen which incorporates low critical temperature quasi-persistent joints was also built. The shielding technique we describe here appears to be especially promising for the realization of large scale high-Tc superconducting screens. [less ▲] Detailed reference viewed: 57 (34 ULg) Modification of the trapped field in bulk HTS as a result of the drilling of a pattern of artificial holes; Fagnard, Jean-François ; Ausloos, Marcel et alin Journal of Physics: Conference Series [=JPCS] (2010), 234 The trapped magnetic field is examined in bulk high-temperature superconductors that are artificially drilled along their c-axis. The influence of the hole pattern on the magnetization is studied and ... [more ▼] The trapped magnetic field is examined in bulk high-temperature superconductors that are artificially drilled along their c-axis. The influence of the hole pattern on the magnetization is studied and compared by means of numerical models and Hall probe mapping techniques. To this aim, we consider two bulk YBCO samples with a rectangular cross-section that are drilled each by six holes arranged either on a rectangular lattice (sample I) or on a centered rectangular lattice (sample II). For the numerical analysis, three different models are considered for calculating the trapped flux: (i), a two-dimensional (2D) Bean model neglecting demagnetizing effects and flux creep, (ii), a 2D finite-element model neglecting demagnetizing effects but incorporating magnetic relaxation in the form of an E – J power law, and, (iii), a 3D finite element analysis that takes into account both the finite height of the sample and flux creep effects. For the experimental analysis, the trapped magnetic flux density is measured above the sample surface by Hall probe mapping performed before and after the drilling process. The maximum trapped flux density in the drilled samples is found to be smaller than that in the plain samples. The smallest magnetization drop is found for sample II, with the centered rectangular lattice. This result is confirmed by the numerical models. In each sample, the relative drops that are calculated independently with the three different models are in good agreement. As observed experimentally, the magnetization drop calculated in the sample II is the smallest one and its relative value is comparable to the measured one. By contrast, the measured magnetization drop in sample (1) is much larger than that predicted by the simulations, most likely because of a change of the microstructure during the drilling process. [less ▲] Detailed reference viewed: 30 (23 ULg) Measurement of dielectric properties at low temperatures: application to the study of magnetoresistive manganite/ insulating oxide bulk compositesVanderbemden, Philippe ; ; et alin Journal of Physics: Conference Series [=JPCS] (2010), 253 In this paper, we report low temperature dielectric measurements of bulk composite electroceramic samples containing a colossal magnetoresistive (CMR) manganite phase (La0.7Ca0.3MnO3 [abbreviated LCMO ... [more ▼] In this paper, we report low temperature dielectric measurements of bulk composite electroceramic samples containing a colossal magnetoresistive (CMR) manganite phase (La0.7Ca0.3MnO3 [abbreviated LCMO]) and an insulating phase (Mn3O4). Details of the experimental system are given and possible experimental artefacts due to moisture are outlined. For a LCMO volume fraction of ~ 16%, the permittivity of the LCMO/ Mn3O4 composite at T = 50 K is found to be much higher than that of pure Mn3O4 and magnetic field dependent. This effect is related to an extrinsic space charge polarization mechanism between the insulating phase (Mn3O4) and the conducting magnetoresistive phase (LCMO). [less ▲] Detailed reference viewed: 39 (21 ULg) Magnetocaloric effect in La0.75Sr0.25MnO3 manganite; ; et al in Journal of Magnetism & Magnetic Materials (2010), 322(21), 3460-3463 The polycrystalline manganite La0.75Sr0.25MnO3 prepared by an alternative carbonate precipitation route reveals the rhombohedral perovskite structure. Magnetization isotherms measured up to 2 T are used ... [more ▼] The polycrystalline manganite La0.75Sr0.25MnO3 prepared by an alternative carbonate precipitation route reveals the rhombohedral perovskite structure. Magnetization isotherms measured up to 2 T are used to determine Curie temperature of 332 K by means of Arrott plot. Maximum of magnetic entropy change is found at Curie temperature. The relative cooling power equal to 64 J/kg for 1.5 T magnetic field, is superior as compared to the manganite with the same chemical composition from the sol–gel method. [less ▲] Detailed reference viewed: 43 (12 ULg) Shielding efficiency and E(J) characteristics measured on large melt cast Bi-2212 hollow cylinders in axial magnetic fieldsFagnard, Jean-François ; ; et alin Superconductor Science and Technology (2010), 23 We show that tubes of melt cast Bi-2212 used as current leads for LTS magnets can also act as efficient magnetic shields. The magnetic screening properties under an axial DC magnetic field are ... [more ▼] We show that tubes of melt cast Bi-2212 used as current leads for LTS magnets can also act as efficient magnetic shields. The magnetic screening properties under an axial DC magnetic field are characterized at several temperatures below the liquid nitrogen temperature (77 K). Two main shielding properties are studied and compared with those of Bi-2223, a material that has been considered in the past for bulk magnetic shields. The first property is related to the maximum magnetic flux density that can be screened, Blim; it is defined as the applied magnetic flux density below which the field attenuation measured at the centre of the shield exceeds 1000. For a cylinder of Bi-2212 with a wall thickness of 5 mm and a large ratio of length over radius, Blim is evaluated to 1 T at T = 10 K. This value largely exceeds the Blim value measured at the same temperature on similar tubes of Bi-2223. The second shielding property that is characterized is the dependence of Blim with respect to variations of the sweep rate of the applied field, dBapp/dt. This dependence is interpreted in terms of the power law E = Ec(J/Jc)^n and allows us to determine the exponent n of this E(J) characteristics for Bi-2212. The characterization of the magnetic field relaxation involves very small values of the electric field. This gives us the opportunity to experimentally determine the E(J) law in an unexplored region of small electric fields. Combining these results with transport and AC shielding measurements, we construct a piecewise E(J) law that spans over 8 orders of magnitude of the electric field. [less ▲] Detailed reference viewed: 53 (34 ULg) Magnetocaloric effect in nano- and polycrystalline manganites La0.5Ca0.5MnO3; ; Fagnard, Jean-François et alin Journal of Alloys & Compounds (2010), 507 Structure, magnetic and magnetocaloric properties of poly- and nanocrystalline La0.5Ca0.5MnO3 manganites prepared by the citrate sol–gel method are studied in a broad temperature range. The Arrott plots ... [more ▼] Structure, magnetic and magnetocaloric properties of poly- and nanocrystalline La0.5Ca0.5MnO3 manganites prepared by the citrate sol–gel method are studied in a broad temperature range. The Arrott plots show that the phase transition is of the second order. The cooling efficiency of 93–97 J/kg is found for the poly- and nanocrystalline samples. The relatively weaker magnetocaloric effect in nanocrystalline La0.5Ca0.5MnO3 is spread over temperature range almost three times broader than for the polycrystalline one. Charge ordering effects decay in manganites with grain sizes below 150 nm. [less ▲] Detailed reference viewed: 54 (14 ULg) Self-heating of bulk high temperature superconductors of finite height subjected to a large alternating magnetic field; Fagnard, Jean-François ; et alin Superconductor Science and Technology (2010), 23 In this work we study, both experimentally and numerically, the self-heating of a bulk, large YBCO pellet of aspect ratio (thickness / diameter) ~ 0.4 subjected to a large AC magnetic field. To ensure ... [more ▼] In this work we study, both experimentally and numerically, the self-heating of a bulk, large YBCO pellet of aspect ratio (thickness / diameter) ~ 0.4 subjected to a large AC magnetic field. To ensure accurate temperature measurements, the sample was placed in an experimental vacuum chamber to achieve a small and reproducible heat transfer coefficient between the superconductor and the cryogenic fluid. The temperature was measured at several locations on the sample surface during the self-heating process. The experimentally determined temperature gradients are found to be very small in this arrangement (< 0.2 K across the radius of the superconductor). The time-dependence of the average temperature T(t) is found to agree well with a theoretical prediction based on the one-dimensional (1-D) Bean model, assuming a uniform temperature in the sample. A 2-D magneto-thermal model was also used to determine the space and time-dependent temperature distribution T(r, z, t) during the application of the AC field. The losses in the bulk pellet were determined using an algorithm based on the numerical method of Brandt, which was combined with a heat diffusion algorithm implemented using a finite-difference method. The model is shown to be able to reproduce the main trends of the observed temperature evolution of the bulk sample during a self-heating process. Finally, the 2-D model is used to study the effect of a non-uniform distribution of critical current density Jc(r, z) on the losses within the bulk superconductor. [less ▲] Detailed reference viewed: 42 (30 ULg) Magneto-thermal phenomena in bulk high temperature superconductors subjected to applied AC magnetic fieldsVanderbemden, Philippe ; Laurent, Philippe ; Fagnard, Jean-François et alin Superconductor Science and Technology (2010), 23 In the present work we study, both theoretically and experimentally, the temperature increase in a bulk high temperature superconductor subjected to applied AC magnetic fields of large amplitude. We ... [more ▼] In the present work we study, both theoretically and experimentally, the temperature increase in a bulk high temperature superconductor subjected to applied AC magnetic fields of large amplitude. We calculate analytically the equilibrium temperatures of the bulk sample as a function of the experimental parameters using a simple critical state model for an infinitely long type-II superconducting slab or cylinder. The results show the existence of a limit heat transfer coefficient (AUlim) separating two thermal regimes with different characteristics. The theoretical analysis predicts a ‘forbidden’ temperature window within which the temperature of the superconductor can never stabilize when the heat transfer coefficient is small. In addition, we determine analytical expressions for two threshold fields Htr1 and Htr2 characterizing the importance of magneto-thermal effects and show that a thermal runaway always occurs when the field amplitude is larger than Htr2. The theoretical predictions of the temperature evolution of the bulk sample during a self-heating process agree well with the experimental data. The simple analytical study presented in this paper enables order of magnitude thermal effects to be estimated for simple superconductor geometries under applied AC magnetic fields and can be used to predict the influence of experimental parameters on the self-heating characteristics of bulk type-II superconductors. [less ▲] Detailed reference viewed: 57 (35 ULg) Local Structure of Mn in (La1-xHox)2/3Ca1/3MnO3 Studied by X-ray Absorption Fine Structure; ; et al in Acta Physica Polonica A (2010), 117(2), 257-261 Results of X-ray absorption fine structure measurements in manganites (La1-xHox)2/3Ca1/3MnO3 with 0.15 < x < 0.50 are presented. When LaMnO3 is doped with a divalent element such as Ca2+, substituting ... [more ▼] Results of X-ray absorption fine structure measurements in manganites (La1-xHox)2/3Ca1/3MnO3 with 0.15 < x < 0.50 are presented. When LaMnO3 is doped with a divalent element such as Ca2+, substituting forLa3+, holes are induced in the filled Mn d orbitals. This leads to a strong ferromagnetic coupling between Mn sites. Ca ions in La1-xCaxMnO3 introduce a distortion of the crystal lattice and mixed valence Mn ions (Mn3+ and Mn4+). On the other hand, in manganites (La1-xHox)2/3Ca1/3MnO3 the substitution of La for Ho causes a lattice distortion and induces a disorder, which reduces a magnetic interaction. The ferromagnetic transition temperature and conductivity decrease very quickly with increasing x. The magnetic and transport properties of compounds depend on the local atomic structure around Mn ions. The information on the bond lengths and Debye–Waller factor are obtained from the extended X-ray absorption fine structure (EXAFS) data analysis. The charge state of Mn is determined from the position of the absorption edge in X-ray absorption near edge structure (XANES) data. XAFS results are in good agreement with magnetic characteristics of the studied materials. [less ▲] Detailed reference viewed: 38 (16 ULg) Pulsed-field magnetization of drilled bulk high-temperature superconductors: flux front propagation in the volume and on the surfaceLousberg, Grégory ; Fagnard, Jean-François ; et alin Superconductor Science and Technology (2009), (22), 125026 We present a method for characterizing the propagation of the magnetic flux in an artificially drilled bulk high-temperature superconductor (HTS) during pulsed-field magnetization. As the magnetic pulse ... [more ▼] We present a method for characterizing the propagation of the magnetic flux in an artificially drilled bulk high-temperature superconductor (HTS) during pulsed-field magnetization. As the magnetic pulse penetrates the cylindrical sample, the magnetic flux density is measured simultaneously in 16 holes by means of microcoils that are placed across the median plane, i.e. at an equal distance from the top and bottom surfaces, and close to the surface of the sample. We discuss the time evolution of the magnetic flux density in the holes during a pulse and measure the time taken by the external magnetic flux to reach each hole. Our data show that the flux front moves faster in the median plane than on the surface when penetrating the sample edge; it then proceeds faster along the surface than in the bulk as it penetrates the sample further. Once the pulse is over, the trapped flux density inside the central hole is found to be about twice as large in the median plane as on the surface. This ratio is confirmed by modelling. [less ▲] Detailed reference viewed: 59 (37 ULg) Magnetic shielding properties of high- Tc superconducting hollow cylinders: model combining experimental data for axial and transverse magnetic field configurationsFagnard, Jean-François ; ; Ausloos, Marcel et alin Superconductor Science and Technology (2009), 22(10), 10500210 Magnetic shielding efficiency was measured on high- Tc superconducting hollow cylinders subjected to either an axial or a transverse magnetic field in a large range of field sweep rates, dBapp/dt. The ... [more ▼] Magnetic shielding efficiency was measured on high- Tc superconducting hollow cylinders subjected to either an axial or a transverse magnetic field in a large range of field sweep rates, dBapp/dt. The behaviour of the superconductor was modelled in order to reproduce the main features of the field penetration curves by using a minimum number of free parameters suitable for both magnetic field orientations. The field penetration measurements were carried out on Pb-doped Bi-2223 tubes at 77 K by applying linearly increasing magnetic fields with a constant sweep rate ranging between 10 uT s[?]1 and 10 mT s[?]1 for both directions of the applied magnetic field. The experimental curves of the internal field versus the applied field, Bin(Bapp), show that, at a given sweep rate, the magnetic field for which the penetration occurs, Blim, is lower for the transverse configuration than for the axial configuration. A power law dependence with large exponent, n', is found between Blim and dBapp/dt. The values of n' are nearly the same for both configurations. We show that the main features of the curves Bin(Bapp) can be reproduced using a simple 2D model, based on the method of Brandt, involving a E(J) power law with an n-exponent and a field-dependent critical current density, Jc(B), (following the Kim model: Jc = Jc0(1+B/B1)[?]1). In particular, a linear relationship between the measured n'-exponents and the n-exponent of the E(J) power law is suggested by taking into account the field dependence of the critical current density. Differences between the axial and the transverse shielding properties can be simply attributed to demagnetizing fields. [less ▲] Detailed reference viewed: 97 (41 ULg) DC and AC Shielding Properties of Bulk High-Tc Superconducting TubesFagnard, Jean-François ; ; Lousberg, Grégory et alin IEEE Transactions on Applied Superconductivity (2009), 19(3), 2905-2908 We have studied numerically and experimentally the magnetic flux penetration in high-Tc superconducting tube subjected to a uniform magnetic field parallel to its long axis. This study is carried in view ... [more ▼] We have studied numerically and experimentally the magnetic flux penetration in high-Tc superconducting tube subjected to a uniform magnetic field parallel to its long axis. This study is carried in view of designing low-frequency magnetic shields by exploiting the diamagnetic properties of high-Tc superconducting ceramics. We have measured the field attenuation for applied magnetic fields in the frequency range 5 mHz-0.1 Hz by Hall probe measurements and at audio frequencies using a sensing coil. A simple 1D analysis using the Kim critical state model was found to be able to reproduce the experimental data satisfactorily. We have also determined the phase shift between the internal and the applied field both experimentally and numerically. Finally, we have studied the sweep rate dependence of the magnetic shielding properties, using data recorded either at several constant sweep rates dB/dt or at several AC fields of various amplitudes and frequencies. Both methods agree with each other and lead to a n -value of the E ~ J n law equal to ~ 40 at 77 K. [less ▲] Detailed reference viewed: 122 (50 ULg) Numerical simulation of the magnetization of high-temperature superconductors: a 3D finite element method using a single time-step iterationLousberg, Grégory ; Ausloos, Marcel ; Geuzaine, Christophe et alin Superconductor Science and Technology (2009), 22 In this paper, we report progress towards a 3D finite element model for the magnetization of a high-temperature superconductor (HTS): we suggest a method that takes into account a power law conductivity ... [more ▼] In this paper, we report progress towards a 3D finite element model for the magnetization of a high-temperature superconductor (HTS): we suggest a method that takes into account a power law conductivity and demagnetization effects, while neglecting the effects associated with currents that are not perpendicular to the local magnetic induction. We consider samples that are subjected to a uniform magnetic field varying linearly with time. Their magnetization is calculated by means of a weak formulation in the magnetostatic approximation of the Maxwell equations (A–φ formulation). An implicit method is used for the temporal resolution (backward Euler scheme) and is solved with the open source solver GetDP. Fixed point iterations are used to deal with the power law conductivity of HTS. The finite element formulation is validated for an HTS tube with large n value by comparing with results obtained with other well-established methods. We show that carrying out the calculations with a single time-step (as opposed to many small time-steps) produces results with excellent accuracy in a drastically reduced simulation time. The numerical method is extended to the study of the trapped magnetization of cylinders that are drilled with different arrays of columnar holes arranged parallel to the cylinder axis. [less ▲] Detailed reference viewed: 136 (51 ULg) Measurement of the magnetic field inside the holes of a drilled bulk high-Tc superconductorLousberg, Grégory ; Fagnard, Jean-François ; et alin Superconductor Science and Technology (2009), 22 We use macroscopic holes drilled in a bulk YBCO superconductor to probe its magnetic properties in the volume of the sample. The sample is subjected to an AC magnetic flux with a density ranging from 30 ... [more ▼] We use macroscopic holes drilled in a bulk YBCO superconductor to probe its magnetic properties in the volume of the sample. The sample is subjected to an AC magnetic flux with a density ranging from 30 to 130 mT and the flux in the superconductor is probed by miniature coils inserted in the holes. In a given hole, three different penetration regimes can be observed: (i) the shielded regime, where no magnetic flux threads the hole; (ii) the gradual penetration regime, where the waveform of the magnetic field has a clipped sine shape whose fundamental component scales with the applied field; and (iii) the flux concentration regime, where the waveform of the magnetic field is nearly a sine wave, with an amplitude exceeding that of the applied field by up to a factor of two. The distribution of the penetration regimes in the holes is compared with that of the magnetic flux density at the top and bottom surfaces of the sample, and is interpreted with the help of optical polarized light micrographs of these surfaces. We show that the measurement of the magnetic field inside the holes can be used as a local characterization of the bulk magnetic properties of the sample. [less ▲] Detailed reference viewed: 114 (80 ULg) Magneto transport characterization of the Sn-doped TbMnO3 manganites; ; Fagnard, Jean-François et alin Journal of Alloys & Compounds (2009), 467(1-2), 35-40 The structural, magnetic and electrical transport properties of the Sn-doped TbMnO3 manganites are studied by X-ray diffraction, ac susceptibility, dc magnetization and electrical resistivity measurements ... [more ▼] The structural, magnetic and electrical transport properties of the Sn-doped TbMnO3 manganites are studied by X-ray diffraction, ac susceptibility, dc magnetization and electrical resistivity measurements. The Sn doping into the Tb and Mn sites of TbMnO3 compresses the unit cell and changes parameters of the antiferromagnetic phase whereas the magnetic moment of Mn are only weakly affected. The electrical resistivity of doped manganites is reduced and the activation energy EA is determined for the thermally activated conduction. [less ▲] Detailed reference viewed: 77 (14 ULg) Magnetotransport of La0.5Ba0.5MnO3; ; Fagnard, Jean-François et alin Journal of Applied Physics (2009), 105(1), 013923-013923-8 Physical properties of polycrystalline La0.5Ba0.5MnO3 are reported from low temperature (10 K) up to above room temperature. An aim has been to obtain microscopic parameters and to search for the ... [more ▼] Physical properties of polycrystalline La0.5Ba0.5MnO3 are reported from low temperature (10 K) up to above room temperature. An aim has been to obtain microscopic parameters and to search for the characteristic lengths in terms of which one can discuss the interplay between magnetic, electric, and phonon excitations. The structural and magnetotransport measurements reveal a set of relatively high transition temperatures (near 300 K) between ferromagnetic/metallic and paramagnetic/semiconducting phases. It is found, in particular, that the so-called localization length increases from 0.085 to 0.24 nm when the magnetic field varies from 0 to 8 T. Moreover a “special field value” ~0.03 T is observed in the description of the electrical resistance. It cannot be presently distinguished whether it is the signature of a spin reorientation transition in the canted phase or a mere saturation field for aligning magnetic domains. The relatively high magnetoresistance effect (~=55% at 8 T and 10 K) makes the La0.5Ba0.5MnO3 a very interesting material for among others sensor applications. [less ▲] Detailed reference viewed: 50 (11 ULg) Magnetic and transport properties of HoMnO3 monocrystals; ; et al in Journal of Optoelectronics and Advanced Materials [= JOAM] (2009), 11 This paper presents results from measurements of the magnetization, specific heat and dielectric constant, and their temperature and magnetic field dependence, for HoMnO3 single crystals. The results are ... [more ▼] This paper presents results from measurements of the magnetization, specific heat and dielectric constant, and their temperature and magnetic field dependence, for HoMnO3 single crystals. The results are discussed in the framework of existing data on magnetic symmetries and the interactions between the Mn-spins, the rare earth moments, and the lattice. From the resulting data, the magnetic phase diagram of HoMnO3 was built. [less ▲] Detailed reference viewed: 50 (9 ULg) Grain boundary effects in bulk colossal magneto resistive (CMR) manganites and manganite/insulator composites: electrical and magnetic propertiesVanderbemden, Philippe ; Vertruyen, Bénédicte ; Ausloos, Marcel et alin Journal of Optoelectronics and Advanced Materials [= JOAM] (2009), 11(9), 1115-1121 In the first part of this paper, we discuss the effects of grain boundaries on the properties of bulk colossal magnetoresistive (CMR) manganites We compare the electrical resistivity and AC magnetic ... [more ▼] In the first part of this paper, we discuss the effects of grain boundaries on the properties of bulk colossal magnetoresistive (CMR) manganites We compare the electrical resistivity and AC magnetic susceptibility of perovskite La-Ca-Mn-O samples with the same nominal stoichiometry but differing in their microstructure (i) a single grain sample, (ii) a sample containing two grains and (iii) a polycrystalline sample Emphasis is placed on information that can be deduced from the measurements in each case In the second part of the paper, we report the data measured on composite samples containing a CMR phase (La-Ca-Mn-O) and an insulating phase (Mn3O4) The results are discussed in the framework of percolation theory We show how the grain boundaries affect the electrical properties of these materials, and we highlight the crucial role of geometric (demagnetization) effects on the resistance vs magnetic field measurements [less ▲] Detailed reference viewed: 78 (23 ULg) STFT-based spectral analysis of urban waterworks leakage detection; ; et al in XIX IMEKO World Congress Proceedings (2009) Water is an essential good for human being necessity. It must be protected against pollution and useless leakage. Urban waterworks is a strategic infrastructure to be managed with particular attention and ... [more ▼] Water is an essential good for human being necessity. It must be protected against pollution and useless leakage. Urban waterworks is a strategic infrastructure to be managed with particular attention and care so that users must be satisfied. Different techniques are used to detect leaks from waterworks, specifically from pipelines carrying water. Among them, spectral analysis is very interesting to apply amid problems related to the pipeline section. This paper presents an application of STFT (short-term Fourier transform) technique for identifying urban waterworks leaks; STFT technique is usually used in processing speech. For the purposes of this research, a specific pipeline plant has been build in other to feature a real case. The pipeline section is almost one inch; the adopted section makes the research very interesting since spectral analysis, based essentially on FFT, is generally used for section greater than 20 cm. [less ▲] Detailed reference viewed: 16 (6 ULg) Influence of microstructure on the thermal conductivity of magnetoresistive La0.7Ca0.3MnO3/Mn3O4 manganite/insulating oxide polycrystalline bulk composites; Vertruyen, Bénédicte ; et alin Journal of Applied Physics (2009), 105(6), 063501 We report the temperature dependence of the thermal conductivity kappa(T) of bulk polycrystalline composite samples containing a magnetoresistive manganite (La0.7Ca0.3MnO3) and an electrically insulating ... [more ▼] We report the temperature dependence of the thermal conductivity kappa(T) of bulk polycrystalline composite samples containing a magnetoresistive manganite (La0.7Ca0.3MnO3) and an electrically insulating phase (Mn3O4). The sample porosity is shown to be a significant parameter affecting the experimental data: after porosity correction the curves display the characteristics of an ideal composite. A fit of the kappa(T) curves at low temperature using the Debye model enables the mean free path of phonons scattered on "boundaries" to be determined. The values are on the order of the grain size but are influenced by the grain arrangement and the presence of twins. [less ▲] Detailed reference viewed: 70 (24 ULg) |
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